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A review of magnesium aluminum chloride complex electrolytes for Mg batteries

Li, Yaqi, Guan, Shaoliang, Huo, Hua, Ma, Yulin, Gao, Yunzhi, Zuo, Pengjian and Yin, Geping 2021. A review of magnesium aluminum chloride complex electrolytes for Mg batteries. Advanced Functional Materials 31 (24) , 2100650. 10.1002/adfm.202100650

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Abstract

Developing suitable electrolytes with high oxidation decomposition potential, low cost, and good compatibility with electrode materials has been a critical challenge in realizing practical magnesium batteries. The emerging magnesium aluminum chloride complex (MACC) electrolytes based on inorganic chloride salts exhibit high Coulombic efficiencies for magnesium batteries. This review summarizes recent studies of MACC electrolytes, focusing on the synthesis, characterization, and chemical environment of Mg species, electrolytic conditioning of electrolytes, and their application in typical magnesium batteries. The electrolyte evolution and influencing factor of electrolytic conditioning are discussed, and several kinds of conditioning-free MACC electrolytes are further introduced. Finally, future trends and perspectives in this field are discussed.

Item Type: Article
Date Type: Publication
Status: Published
Schools: Chemistry
Cardiff Catalysis Institute (CCI)
Publisher: Wiley
ISSN: 1616-301X
Date of First Compliant Deposit: 18 August 2021
Date of Acceptance: 31 March 2021
Last Modified: 13 May 2022 21:53
URI: https://orca.cardiff.ac.uk/id/eprint/143514

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