Lezcano-González, Inés, Cong, Peixi, Campbell, Emma, Panchal, Monik, Agote-Arán, Miren, Celorrio, Verónica, He, Qian  ORCID: https://orcid.org/0000-0003-4891-3581, Oord, Ramon, Weckhuysen, Bert M. and Beale, Andrew M.
2022.
Structure-activity relationships in highly active Platinum-Tin MFI-type Zeolite catalysts for propane dehydrogenation.
ChemCatChem
14
(7)
, e202101828.
10.1002/cctc.202101828
|
Preview |
PDF
- Published Version
Available under License Creative Commons Attribution. Download (898kB) | Preview |
Official URL: http://dx.doi.org/10.1002/cctc.202101828
Abstract
Pt/Sn-containing MFI zeolites prepared by one-pot hydrothermal methods are highly active and selective catalysts for propane dehydrogenation. An alternative preparation method is reported alongside an in-depth characterization of Pt and Sn before and after reaction. Pt species dispersed on highly-defective Silicalite-1 show a significantly long catalytic lifetime with an improved coke resistance, but increased Pt−Sn alloying and the (eventual) build-up of carbon leads to deactivation.
| Item Type: | Article |
|---|---|
| Date Type: | Publication |
| Status: | Published |
| Schools: | Schools > Chemistry Research Institutes & Centres > Cardiff Catalysis Institute (CCI) |
| Additional Information: | This is an open access article under the terms of the Creative Commons Attribution License. This article also appears in: Society Volumes: The Netherlands. |
| Publisher: | Wiley-VCH Verlag |
| ISSN: | 1867-3880 |
| Funders: | EPSRC |
| Date of First Compliant Deposit: | 10 March 2022 |
| Date of Acceptance: | 28 January 2022 |
| Last Modified: | 23 May 2023 14:05 |
| URI: | https://orca.cardiff.ac.uk/id/eprint/148236 |
Citation Data
Cited 4 times in Scopus. View in Scopus. Powered By Scopus® Data
Actions (repository staff only)
 |
Edit Item |
Dimensions
Dimensions