Lezcano-González, Inés, Cong, Peixi, Campbell, Emma, Panchal, Monik, Agote-Arán, Miren, Celorrio, Verónica, He, Qian ORCID: https://orcid.org/0000-0003-4891-3581, Oord, Ramon, Weckhuysen, Bert M. and Beale, Andrew M. 2022. Structure-activity relationships in highly active Platinum-Tin MFI-type Zeolite catalysts for propane dehydrogenation. ChemCatChem 14 (7) , e202101828. 10.1002/cctc.202101828 |
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Official URL: http://dx.doi.org/10.1002/cctc.202101828
Abstract
Pt/Sn-containing MFI zeolites prepared by one-pot hydrothermal methods are highly active and selective catalysts for propane dehydrogenation. An alternative preparation method is reported alongside an in-depth characterization of Pt and Sn before and after reaction. Pt species dispersed on highly-defective Silicalite-1 show a significantly long catalytic lifetime with an improved coke resistance, but increased Pt−Sn alloying and the (eventual) build-up of carbon leads to deactivation.
Item Type: | Article |
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Date Type: | Publication |
Status: | Published |
Schools: | Chemistry Cardiff Catalysis Institute (CCI) |
Additional Information: | This is an open access article under the terms of the Creative Commons Attribution License. This article also appears in: Society Volumes: The Netherlands. |
Publisher: | Wiley-VCH Verlag |
ISSN: | 1867-3880 |
Funders: | EPSRC |
Date of First Compliant Deposit: | 10 March 2022 |
Date of Acceptance: | 28 January 2022 |
Last Modified: | 23 May 2023 14:05 |
URI: | https://orca.cardiff.ac.uk/id/eprint/148236 |
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